CORDIS Project
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This project investigates the mechanisms of hydrogen atom abstraction and hydride transfer in chemical reactions, focusing on enzymatic selectivity. It aims to develop a thermodynamic model to enhance the understanding of these processes for applications in carbon dioxide reduction and bond activation.
The crucial step for selective cleavage and formation of C-H bonds is a concerted transfer of proton (PT) and electron(s) (ET): hydrogen atom abstraction (HAA) or hydride transfer (HT).
The HAA and HT processes can be employed to various chemical transformations: from activation of inert bonds to reduction of CO2.
This approach, however, requires a strict control of the regioselectivity of the reaction.
Notably, enzymes - catalysts developed by Nature, are characterised by high activity and sele…
USTAV FYZIKALNI CHEMIE J. HEYROVSKEHO AV CR, v. v. i.
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