CORDIS Project
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This project introduces a method for the selective transformation of tertiary amines using a combination of three molecular catalysts. By employing visible light, the process enhances the production of desired amine enantiomers while minimizing waste, making it a sustainable approach for synthetic organic chemistry.
A method is proposed for the deracemisation of tertiary amines via the joint action of three distinct molecular catalysts - an Ir(III) photocatalyst, a chiral Brønsted base and a chiral thiol hydrogen-atom transfer additive.
Through sequential visible-light driven electron transfer (ET), proton transfer (PT) and hydrogen-atom transfer (HAT), proximal stereocentres to amine functional groups can be selectively targeted for destruction of the undesired substrate enantiomer, and restored as the de…
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United States, Princeton, Nj
Type: University / higher education
Activity type: Higher or Secondary Education Establishments
SME: No
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