CORDIS Project
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The project aims to generate cyclopropylacyl radicals from xanthates, which can lead to valuable cyclopropyl ketones for organic synthesis. It will explore their unique reactivity and apply these findings to synthesize the natural product (+)-Ineleganolide.
Preliminary work in the Zard's group has shown that cyclopropylacyl radicals can be generated from the corresponding xanthates.
These unique species do not easily undergo decarbonylation or ring opening processes.
These features can be exploited because the products, cyclopropyl ketones, have been found to be exceptional substrates in organic synthesis.
Additionally, control of the decarbonylation and/or ring-opening processes can be combined with the powerful nature of the xanthate transfe…
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